IndiumV3, Russie, Analysis, bibRecord, 000026

Ce2PdIng, Ce3PdIn11 and Ce5Pd2In19-members of homological series based on AuCu3- and PtHg2-type structural units

Identifieur interne : 000026 ( Russie/Analysis ); précédent : 000025; suivant : 000027

Ce2PdIng, Ce3PdIn11 and Ce5Pd2In19-members of homological series based on AuCu3- and PtHg2-type structural units

Auteurs : RBID : Pascal:13-0190075

Descripteurs français

Pascal (Inist)
- Motif structural, Structure cristalline, Diffraction RX, Groupe espace, Paramètre cristallin, Propriété électrique, Propriété transport, Phénomène transport, Loi Curie Weiss, Résistivité électrique, Conductivité électrique, Dépendance température, Spin flip, Interaction échange, Monocristal, Cérium alliage, Palladium alliage, Indium alliage, Matériau paramagnétique, Effet Kondo, Composé intermétallique, Propriété magnétique, Corrélation forte, Corrélation électronique, Réseau Kondo, CeIn3, 6166, 7215Q.

English descriptors

KwdEn :
- Cerium alloys, Crystal structure, Curie-Weiss law, Electric resistivity, Electrical conductivity, Electrical properties, Electron correlations, Exchange interactions, Indium alloys, Intermetallic compounds, Kondo effect, Kondo lattice, Lattice parameters, Magnetic properties, Monocrystals, Palladium alloys, Paramagnetic materials, Space groups, Spin flip, Strong correlation, Structural unit, Temperature dependence, Transport processes, Transport properties, XRD.

Abstract

Crystal structures of three members of a unique homological series with the general formula Ce_mPd_nIn_3m+2n based on the AuCu₃ and PtHg₂ structure types were studied by single-crystal X-ray diffraction. The compounds crystallize with space group P4/mmm (Z=1) and the lattice parameters: a=4.6900(9) Å, c=12.185(6) Å for Ce₂PdIn₈, a=4.6846(8) A, c=16.846(8)A for Ce₃PdIn₁₁, and a=4.70120(10) Å, c=29.7359(4) Å for Ce₅Pd₂In₁₉. The crystal structures of Ce₃PdIn₁₁ and Ce₅Pd₂In₁₉ represent new types. The three structures constitute of [CeIn₃] cuboctahedra layers and [PdIn₂] rectangular polyhedra layers, alternating along the tetragonal c-axis in accordance with the m:n proportion. The magnetic and electrical transport properties of the novel compounds Ce₃PdIn₁₁ and Ce₅Pd₂In₁₉ were investigated down to 1.72 K. Both indides are Curie-Weiss paramagnets due to the presence of fairly well localized 4f electrons of trivalent cerium ions. The electrical resistivity of both materials is dominated over an extended temperature range by strong spin-flip Kondo interactions with the characteristic temperature scale of 20-30 K.

Links toward previous steps (curation, corpus...)

to stream Main, to step Corpus: 000D41
to stream Main, to step Repository: 001084
to stream Russie, to step Extraction: 000026

Links to Exploration step

Pascal:13-0190075

Le document en format XML

<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en" level="a">Ce<sub>2</sub>
PdIng, Ce<sub>3</sub>
PdIn<sub>11</sub>
 and Ce<sub>5</sub>
Pd<sub>2</sub>
In<sub>19</sub>
-members of homological series based on AuCu<sub>3</sub>
<sup>-</sup>
 and PtHg<sub>2</sub>
-type structural units</title>
<author><name sortKey="Tursina, A" uniqKey="Tursina A">A. Tursina</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Department of Chemistry, Lomonosov Moscow State University</s1>
<s2>Moscow 119991</s2>
<s3>RUS</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
</inist:fA14>
<country>Russie</country>
<placeName><settlement type="city">Moscou</settlement>
<region>District fédéral central</region>
</placeName>
</affiliation>
</author>
<author><name sortKey="Nesterenko, S" uniqKey="Nesterenko S">S. Nesterenko</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Department of Chemistry, Lomonosov Moscow State University</s1>
<s2>Moscow 119991</s2>
<s3>RUS</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
</inist:fA14>
<country>Russie</country>
<placeName><settlement type="city">Moscou</settlement>
<region>District fédéral central</region>
</placeName>
</affiliation>
</author>
<author><name sortKey="Seropegin, Y" uniqKey="Seropegin Y">Y. Seropegin</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Department of Chemistry, Lomonosov Moscow State University</s1>
<s2>Moscow 119991</s2>
<s3>RUS</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
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<country>Russie</country>
<placeName><settlement type="city">Moscou</settlement>
<region>District fédéral central</region>
</placeName>
</affiliation>
</author>
<author><name sortKey="Noel, H" uniqKey="Noel H">H. Noël</name>
<affiliation wicri:level="4"><inist:fA14 i1="02"><s1>Laboratoire de Chimie du Solide et Matériaux, UMR6226 CNRS-Université de Rennes 1, Avenue du Général Leclerc</s1>
<s2>Rennes 30542</s2>
<s3>FRA</s3>
<sZ>4 aut.</sZ>
</inist:fA14>
<country>France</country>
<placeName><region type="region" nuts="2">Languedoc-Roussillon</region>
</placeName>
<orgName type="university">Université de Rennes 1</orgName>
</affiliation>
</author>
<author><name sortKey="Kaczorowski, D" uniqKey="Kaczorowski D">D. Kaczorowski</name>
<affiliation wicri:level="1"><inist:fA14 i1="03"><s1>Institute of Low Temperature and Structure Research, Polish Academy of Sciences, P.O.Box 1410</s1>
<s2>Wroclaw 50-950</s2>
<s3>POL</s3>
<sZ>5 aut.</sZ>
</inist:fA14>
<country>Pologne</country>
<wicri:noRegion>Wroclaw 50-950</wicri:noRegion>
</affiliation>
</author>
</titleStmt>
<publicationStmt><idno type="inist">13-0190075</idno>
<date when="2013">2013</date>
<idno type="stanalyst">PASCAL 13-0190075 INIST</idno>
<idno type="RBID">Pascal:13-0190075</idno>
<idno type="wicri:Area/Main/Corpus">000D41</idno>
<idno type="wicri:Area/Main/Repository">001084</idno>
<idno type="wicri:Area/Russie/Extraction">000026</idno>
</publicationStmt>
<seriesStmt><idno type="ISSN">0022-4596</idno>
<title level="j" type="abbreviated">J. solid state chem. : (Print)</title>
<title level="j" type="main">Journal of solid state chemistry : (Print)</title>
</seriesStmt>
</fileDesc>
<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Cerium alloys</term>
<term>Crystal structure</term>
<term>Curie-Weiss law</term>
<term>Electric resistivity</term>
<term>Electrical conductivity</term>
<term>Electrical properties</term>
<term>Electron correlations</term>
<term>Exchange interactions</term>
<term>Indium alloys</term>
<term>Intermetallic compounds</term>
<term>Kondo effect</term>
<term>Kondo lattice</term>
<term>Lattice parameters</term>
<term>Magnetic properties</term>
<term>Monocrystals</term>
<term>Palladium alloys</term>
<term>Paramagnetic materials</term>
<term>Space groups</term>
<term>Spin flip</term>
<term>Strong correlation</term>
<term>Structural unit</term>
<term>Temperature dependence</term>
<term>Transport processes</term>
<term>Transport properties</term>
<term>XRD</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr"><term>Motif structural</term>
<term>Structure cristalline</term>
<term>Diffraction RX</term>
<term>Groupe espace</term>
<term>Paramètre cristallin</term>
<term>Propriété électrique</term>
<term>Propriété transport</term>
<term>Phénomène transport</term>
<term>Loi Curie Weiss</term>
<term>Résistivité électrique</term>
<term>Conductivité électrique</term>
<term>Dépendance température</term>
<term>Spin flip</term>
<term>Interaction échange</term>
<term>Monocristal</term>
<term>Cérium alliage</term>
<term>Palladium alliage</term>
<term>Indium alliage</term>
<term>Matériau paramagnétique</term>
<term>Effet Kondo</term>
<term>Composé intermétallique</term>
<term>Propriété magnétique</term>
<term>Corrélation forte</term>
<term>Corrélation électronique</term>
<term>Réseau Kondo</term>
<term>CeIn3</term>
<term>6166</term>
<term>7215Q</term>
</keywords>
</textClass>
</profileDesc>
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<front><div type="abstract" xml:lang="en">Crystal structures of three members of a unique homological series with the general formula Ce<sub>m</sub>
Pd<sub>n</sub>
In<sub>3m+2n</sub>
 based on the AuCu<sub>3</sub>
 and PtHg<sub>2</sub>
 structure types were studied by single-crystal X-ray diffraction. The compounds crystallize with space group P4/mmm (Z=1) and the lattice parameters: a=4.6900(9) Å, c=12.185(6) Å for Ce<sub>2</sub>
PdIn<sub>8</sub>
, a=4.6846(8) A, c=16.846(8)A for Ce<sub>3</sub>
PdIn<sub>11</sub>
, and a=4.70120(10) Å, c=29.7359(4) Å for Ce<sub>5</sub>
Pd<sub>2</sub>
In<sub>19</sub>
. The crystal structures of Ce<sub>3</sub>
PdIn<sub>11</sub>
 and Ce<sub>5</sub>
Pd<sub>2</sub>
In<sub>19</sub>
 represent new types. The three structures constitute of [CeIn<sub>3</sub>
] cuboctahedra layers and [PdIn<sub>2</sub>
] rectangular polyhedra layers, alternating along the tetragonal c-axis in accordance with the m:n proportion. The magnetic and electrical transport properties of the novel compounds Ce<sub>3</sub>
PdIn<sub>11</sub>
 and Ce<sub>5</sub>
Pd<sub>2</sub>
In<sub>19</sub>
 were investigated down to 1.72 K. Both indides are Curie-Weiss paramagnets due to the presence of fairly well localized 4f electrons of trivalent cerium ions. The electrical resistivity of both materials is dominated over an extended temperature range by strong spin-flip Kondo interactions with the characteristic temperature scale of 20-30 K.</div>
</front>
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<fA03 i2="1"><s0>J. solid state chem. : (Print)</s0>
</fA03>
<fA05><s2>200</s2>
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<fA08 i1="01" i2="1" l="ENG"><s1>Ce<sub>2</sub>
PdIng, Ce<sub>3</sub>
PdIn<sub>11</sub>
 and Ce<sub>5</sub>
Pd<sub>2</sub>
In<sub>19</sub>
-members of homological series based on AuCu<sub>3</sub>
<sup>-</sup>
 and PtHg<sub>2</sub>
-type structural units</s1>
</fA08>
<fA11 i1="01" i2="1"><s1>TURSINA (A.)</s1>
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<fA11 i1="02" i2="1"><s1>NESTERENKO (S.)</s1>
</fA11>
<fA11 i1="03" i2="1"><s1>SEROPEGIN (Y.)</s1>
</fA11>
<fA11 i1="04" i2="1"><s1>NOËL (H.)</s1>
</fA11>
<fA11 i1="05" i2="1"><s1>KACZOROWSKI (D.)</s1>
</fA11>
<fA14 i1="01"><s1>Department of Chemistry, Lomonosov Moscow State University</s1>
<s2>Moscow 119991</s2>
<s3>RUS</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
</fA14>
<fA14 i1="02"><s1>Laboratoire de Chimie du Solide et Matériaux, UMR6226 CNRS-Université de Rennes 1, Avenue du Général Leclerc</s1>
<s2>Rennes 30542</s2>
<s3>FRA</s3>
<sZ>4 aut.</sZ>
</fA14>
<fA14 i1="03"><s1>Institute of Low Temperature and Structure Research, Polish Academy of Sciences, P.O.Box 1410</s1>
<s2>Wroclaw 50-950</s2>
<s3>POL</s3>
<sZ>5 aut.</sZ>
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<fA20><s1>7-12</s1>
</fA20>
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<fA66 i1="01"><s0>NLD</s0>
</fA66>
<fC01 i1="01" l="ENG"><s0>Crystal structures of three members of a unique homological series with the general formula Ce<sub>m</sub>
Pd<sub>n</sub>
In<sub>3m+2n</sub>
 based on the AuCu<sub>3</sub>
 and PtHg<sub>2</sub>
 structure types were studied by single-crystal X-ray diffraction. The compounds crystallize with space group P4/mmm (Z=1) and the lattice parameters: a=4.6900(9) Å, c=12.185(6) Å for Ce<sub>2</sub>
PdIn<sub>8</sub>
, a=4.6846(8) A, c=16.846(8)A for Ce<sub>3</sub>
PdIn<sub>11</sub>
, and a=4.70120(10) Å, c=29.7359(4) Å for Ce<sub>5</sub>
Pd<sub>2</sub>
In<sub>19</sub>
. The crystal structures of Ce<sub>3</sub>
PdIn<sub>11</sub>
 and Ce<sub>5</sub>
Pd<sub>2</sub>
In<sub>19</sub>
 represent new types. The three structures constitute of [CeIn<sub>3</sub>
] cuboctahedra layers and [PdIn<sub>2</sub>
] rectangular polyhedra layers, alternating along the tetragonal c-axis in accordance with the m:n proportion. The magnetic and electrical transport properties of the novel compounds Ce<sub>3</sub>
PdIn<sub>11</sub>
 and Ce<sub>5</sub>
Pd<sub>2</sub>
In<sub>19</sub>
 were investigated down to 1.72 K. Both indides are Curie-Weiss paramagnets due to the presence of fairly well localized 4f electrons of trivalent cerium ions. The electrical resistivity of both materials is dominated over an extended temperature range by strong spin-flip Kondo interactions with the characteristic temperature scale of 20-30 K.</s0>
</fC01>
<fC02 i1="01" i2="3"><s0>001B60A66</s0>
</fC02>
<fC02 i1="02" i2="3"><s0>001B70B15Q</s0>
</fC02>
<fC03 i1="01" i2="X" l="FRE"><s0>Motif structural</s0>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="ENG"><s0>Structural unit</s0>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="SPA"><s0>Motivo estructural</s0>
<s5>01</s5>
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<fC03 i1="02" i2="3" l="FRE"><s0>Structure cristalline</s0>
<s5>02</s5>
</fC03>
<fC03 i1="02" i2="3" l="ENG"><s0>Crystal structure</s0>
<s5>02</s5>
</fC03>
<fC03 i1="03" i2="3" l="FRE"><s0>Diffraction RX</s0>
<s5>03</s5>
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<fC03 i1="03" i2="3" l="ENG"><s0>XRD</s0>
<s5>03</s5>
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<fC03 i1="04" i2="3" l="FRE"><s0>Groupe espace</s0>
<s5>04</s5>
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<fC03 i1="04" i2="3" l="ENG"><s0>Space groups</s0>
<s5>04</s5>
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<fC03 i1="05" i2="3" l="FRE"><s0>Paramètre cristallin</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="3" l="ENG"><s0>Lattice parameters</s0>
<s5>05</s5>
</fC03>
<fC03 i1="06" i2="3" l="FRE"><s0>Propriété électrique</s0>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="3" l="ENG"><s0>Electrical properties</s0>
<s5>06</s5>
</fC03>
<fC03 i1="07" i2="X" l="FRE"><s0>Propriété transport</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="X" l="ENG"><s0>Transport properties</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="X" l="SPA"><s0>Propiedad transporte</s0>
<s5>07</s5>
</fC03>
<fC03 i1="08" i2="3" l="FRE"><s0>Phénomène transport</s0>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="3" l="ENG"><s0>Transport processes</s0>
<s5>08</s5>
</fC03>
<fC03 i1="09" i2="3" l="FRE"><s0>Loi Curie Weiss</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="3" l="ENG"><s0>Curie-Weiss law</s0>
<s5>09</s5>
</fC03>
<fC03 i1="10" i2="3" l="FRE"><s0>Résistivité électrique</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="3" l="ENG"><s0>Electric resistivity</s0>
<s5>10</s5>
</fC03>
<fC03 i1="11" i2="3" l="FRE"><s0>Conductivité électrique</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="3" l="ENG"><s0>Electrical conductivity</s0>
<s5>11</s5>
</fC03>
<fC03 i1="12" i2="3" l="FRE"><s0>Dépendance température</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="3" l="ENG"><s0>Temperature dependence</s0>
<s5>12</s5>
</fC03>
<fC03 i1="13" i2="3" l="FRE"><s0>Spin flip</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="3" l="ENG"><s0>Spin flip</s0>
<s5>13</s5>
</fC03>
<fC03 i1="14" i2="3" l="FRE"><s0>Interaction échange</s0>
<s5>14</s5>
</fC03>
<fC03 i1="14" i2="3" l="ENG"><s0>Exchange interactions</s0>
<s5>14</s5>
</fC03>
<fC03 i1="15" i2="3" l="FRE"><s0>Monocristal</s0>
<s5>15</s5>
</fC03>
<fC03 i1="15" i2="3" l="ENG"><s0>Monocrystals</s0>
<s5>15</s5>
</fC03>
<fC03 i1="16" i2="3" l="FRE"><s0>Cérium alliage</s0>
<s5>16</s5>
</fC03>
<fC03 i1="16" i2="3" l="ENG"><s0>Cerium alloys</s0>
<s5>16</s5>
</fC03>
<fC03 i1="17" i2="3" l="FRE"><s0>Palladium alliage</s0>
<s5>17</s5>
</fC03>
<fC03 i1="17" i2="3" l="ENG"><s0>Palladium alloys</s0>
<s5>17</s5>
</fC03>
<fC03 i1="18" i2="3" l="FRE"><s0>Indium alliage</s0>
<s5>18</s5>
</fC03>
<fC03 i1="18" i2="3" l="ENG"><s0>Indium alloys</s0>
<s5>18</s5>
</fC03>
<fC03 i1="19" i2="3" l="FRE"><s0>Matériau paramagnétique</s0>
<s5>19</s5>
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<fC03 i1="19" i2="3" l="ENG"><s0>Paramagnetic materials</s0>
<s5>19</s5>
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<fC03 i1="20" i2="3" l="FRE"><s0>Effet Kondo</s0>
<s5>29</s5>
</fC03>
<fC03 i1="20" i2="3" l="ENG"><s0>Kondo effect</s0>
<s5>29</s5>
</fC03>
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<s5>30</s5>
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<s5>30</s5>
</fC03>
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<s5>31</s5>
</fC03>
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<s5>31</s5>
</fC03>
<fC03 i1="23" i2="3" l="FRE"><s0>Corrélation forte</s0>
<s5>32</s5>
</fC03>
<fC03 i1="23" i2="3" l="ENG"><s0>Strong correlation</s0>
<s5>32</s5>
</fC03>
<fC03 i1="24" i2="3" l="FRE"><s0>Corrélation électronique</s0>
<s5>33</s5>
</fC03>
<fC03 i1="24" i2="3" l="ENG"><s0>Electron correlations</s0>
<s5>33</s5>
</fC03>
<fC03 i1="25" i2="X" l="FRE"><s0>Réseau Kondo</s0>
<s5>34</s5>
</fC03>
<fC03 i1="25" i2="X" l="ENG"><s0>Kondo lattice</s0>
<s5>34</s5>
</fC03>
<fC03 i1="25" i2="X" l="SPA"><s0>Red Kondo</s0>
<s5>34</s5>
</fC03>
<fC03 i1="26" i2="3" l="FRE"><s0>CeIn3</s0>
<s4>INC</s4>
<s5>46</s5>
</fC03>
<fC03 i1="27" i2="3" l="FRE"><s0>6166</s0>
<s4>INC</s4>
<s5>71</s5>
</fC03>
<fC03 i1="28" i2="3" l="FRE"><s0>7215Q</s0>
<s4>INC</s4>
<s5>72</s5>
</fC03>
<fN21><s1>175</s1>
</fN21>
<fN44 i1="01"><s1>OTO</s1>
</fN44>
<fN82><s1>OTO</s1>
</fN82>
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{{Explor lien
   |wiki=   *** parameter Area/wikiCode missing *** 
   |area=    IndiumV3
   |flux=    Russie
   |étape=   Analysis
   |type=    RBID
   |clé=     Pascal:13-0190075
   |texte=   Ce2PdIng, Ce3PdIn11 and Ce5Pd2In19-members of homological series based on AuCu3- and PtHg2-type structural units
}}

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Ce2PdIng, Ce3PdIn11 and Ce5Pd2In19-members of homological series based on AuCu3- and PtHg2-type structural units

Ce2PdIng, Ce3PdIn11 and Ce5Pd2In19-members of homological series based on AuCu3- and PtHg2-type structural units

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